If you are just sitting on money to burn, I don't see anything wrong with buying an unlock pack or two. However, be aware that it's quite easy to unlock the skills yourself for free (quests, buying skills from trainers, unlocking skills with faction).
If you're going to buy an unlock pack, I recommend a weapons/mods pack over a skill pack. Unlocking all the mods (or identifying them) is quite tedious, and a pack lets you use faction to unlock skills (buying one pack instead of however many there are now).
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